Catalyst-Free Construction of Imidazole-Pyrrolo[1,2-a]pyrazine Hybrid, 2,6-Disubstituted Imidazo[1,2-a]pyrrolo[2,1-c]pyrazine via Regioselective Annulative Functionalizations
  • Oh, Hyunjin
  • 구도희
  • Jung, Myungho
  • Lee, Sunhee
  • Kim, Ikyon
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초록

Highly efficient catalyst-free annulative functionalization approaches to a novel imidazole-pyrrolo[1,2-a]pyrazine hybrid structure were devised from the reaction of beta-enaminone with propargylamine where regioselective conjugate substitution of beta-enaminone with propargylamine followed by cycloisomerization proceeded smoothly in a domino fashion to construct two heterocyclic moieties (pyrazine and imidazole) via successive formation of three C-N bonds, leading to the target tricyclic skeleton.

제목
Catalyst-Free Construction of Imidazole-Pyrrolo[1,2-a]pyrazine Hybrid, 2,6-Disubstituted Imidazo[1,2-a]pyrrolo[2,1-c]pyrazine via Regioselective Annulative Functionalizations
저자
Oh, Hyunjin구도희Jung, MyunghoLee, SunheeKim, Ikyon
DOI
10.1021/acs.joc.4c01576
발행일
2024-12
저널명
Journal of Organic Chemistry
89
24
페이지
17966 ~ 17990