Anisotropic magnetic properties and giant rotating magnetocaloric effect in double-perovskite Tb2CoMnO6
- Authors
- Moon, J. Y.; Kim, M. K.; Oh, D. G.; Kim, J. H.; Shin, H. J.; Choi, Y. J.; Lee, N.
- Issue Date
- Nov-2018
- Publisher
- AMER PHYSICAL SOC
- Keywords
- Magnetocaloric effect; Double perovskites
- Citation
- PHYSICAL REVIEW B, v.98, no.17
- Journal Title
- PHYSICAL REVIEW B
- Volume
- 98
- Number
- 17
- URI
- https://yscholarhub.yonsei.ac.kr/handle/2021.sw.yonsei/6638
- DOI
- 10.1103/PhysRevB.98.174424
- ISSN
- 2469-9950
2469-9969
- Abstract
- We investigated the anisotropy of the magnetic and magnetocaloric properties of single-crystalline double-perovskite Tb2CoMnO6, which crystallizes in a monoclinic P2(1)/n structure. Due to dissimilar magnetic anisotropy, the ferromagnetic order of the Co2+ and Mn4+ moments emerges along the c axis at T-C = 100 K, and the larger Tb3+ moments align perpendicular to the c axis, below T-Tb = 15 K. The intricate temperature development of the metamagnetism along the c axis results in a large negative change in the magnetic entropy at low temperature. On the other hand, the larger but almost reversible magnetization, perpendicular to the c axis, results in a small and positive entropy change. This highly anisotropic magnetocaloric effect (MCE) leads to a giant rotational MCE, estimated to be 20.8 J/kg K. Our findings, based on the magnetic anisotropy in Tb2CoMnO6, enrich fundamental and applied research on magnetic materials, considering the distinct magnetic characteristics of double perovskites.
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Collections - College of Science > Physics > 1. Journal Articles
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